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GUI Odyssey is an extensive dataset for training and evaluating cross‑application navigation agents on mobile devices. It contains 7,735 episodes collected from six types of mobile devices, covering six cross‑application task types, 201 apps, and 1.4 K app combinations. The data structure includes episode ID, device info, task info, total step count, and detailed step records. The dataset supports multiple split strategies—random, task, device, and app splits—to assess agent performance under various conditions. It is released under the Creative Commons Attribution 4.0 International License.